Covalent POM-Ir hybrid assemblies: tuning redox properties for light-driven multiple charge accumulation
Résumé
This study reports the synthesis, electrochemical characterization, and photophysical properties of two novel photoactive polyoxometalate (POM)-Ir photosensitizer hybrid assemblies. Under visible light irradiation in the presence of triethylamine and trifluoroacetic acid, the polyoxomolybdate-based dyad photoaccumulates the electrons via an efficient intramolecular photoinduced electron transfer process.
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