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Tensor Network Simulation of Non-Markovian Dynamics in Organic Polaritons

Abstract : We calculate the exact many-body time dynamics of polaritonic states supported by an optical cavity filled with organic molecules. Optical, vibrational, and radiative processes are treated on an equal footing employing the time-dependent variational matrix product states algorithm. We demonstrate signatures of non-Markovian vibronic dynamics and its fingerprints in the far-field photon emission spectrum at arbitrary light-matter interaction scales, ranging from the weak to the strong coupling regimes. We analyze both the single-and many-molecule cases, showing the crucial role played by the collective motion of molecular nuclei and dark states in determining the polariton dynamics and the subsequent photon emission.
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Submitted on : Saturday, November 23, 2019 - 8:35:26 PM
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Javier del Pino, Florian A. y. N. Schröder, Alex W Chin, Johannes Feist, Francisco J Garcia-Vidal. Tensor Network Simulation of Non-Markovian Dynamics in Organic Polaritons. Physical Review Letters, American Physical Society, 2018, 121 (22), ⟨10.1103/PhysRevLett.121.227401⟩. ⟨hal-02377564⟩



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