Process tensor approaches to modeling two-dimensional spectroscopy - Sorbonne Université
Pré-Publication, Document De Travail Année : 2024

Process tensor approaches to modeling two-dimensional spectroscopy

Résumé

Problems in the field of open quantum systems often involve an environment that strongly influences the dynamics of excited states. Here we present a numerical method to model optical spectra of non-Markovian open quantum systems. The method employs a process tensor framework to efficiently compute multi-time correlations in a numerically exact way. To demonstrate the efficacy of our method, we compare 2D electronic spectroscopy simulations produced through our method to Markovian master equation simulations in three different system-bath coupling regimes.
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Dates et versions

hal-04796901 , version 1 (21-11-2024)

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Roosmarijn de Wit, Jonathan Keeling, Brendon W. Lovett, Alex W. Chin. Process tensor approaches to modeling two-dimensional spectroscopy. 2024. ⟨hal-04796901⟩
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