From Enynyl Esters to Functionalized Polycyclic Derivatives via Cycloisomerization and Post-Functionalization
Abstract
The post-functionalization of ketone products originating from the PtCl2-catalyzed cycloisomerization of enynyl esters is described. Postfunctionalization has been accomplished via diastereoselective alkylation, regioselective cyclopropane opening and regioselective Baeyer Villiger and Beckmann rearrangements to provide functionalized polycycles.
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