Probing the Fluorescence Dipoles of Single Cubic CdSe/CdS Nanoplatelets with Vertical or Horizontal Orientations - Sorbonne Université
Article Dans Une Revue ACS photonics Année : 2018

Probing the Fluorescence Dipoles of Single Cubic CdSe/CdS Nanoplatelets with Vertical or Horizontal Orientations

Résumé

Measuring the orientation of a single fluorescent nanoemitter and obtaining emitters with a desired orientation is of highest importance for nanophotonics, especially in plasmonics where an emitting dipole close to a metallic surface will couple efficiently to plasmonic modes only if it is deposited vertically. Control of the orientation of a nano-object remains a challenge. Achieving vertical orientation, or having an information on the dipole orientation are key steps for efficient plasmonic excitation. We consider here cubic-shaped nanoplatelets with a thin CdSe core sandwiched in a thick CdS shell. By a combination of polarization measurement and radiation pattern Fourier analysis, we show that each single platelet behaves with excellent precision as a 2D dipole (sum of 2 orthogonal incoherent dipoles) and having only two possible orientations: either they lie horizontally on the substrate or they stand vertically on the edge. The cubic shape allows some platelets to deposit vertically so that they present a deterministic vertical dipole component.

Domaines

Chimie
Fichier principal
Vignette du fichier
Probing the fluorescence dipoles of single cubic CdSeCdS nanoplatelets with vertical or horizontal orientations revised.pdf (1.04 Mo) Télécharger le fichier
Origine Fichiers produits par l'(les) auteur(s)
Loading...

Dates et versions

hal-01777981 , version 1 (25-04-2018)

Identifiants

Citer

Fu Feng, Loan Thu Nguyen, Michel Nasilowski, Brice Nadal, Benoît Dubertret, et al.. Probing the Fluorescence Dipoles of Single Cubic CdSe/CdS Nanoplatelets with Vertical or Horizontal Orientations. ACS photonics, 2018, 5 ( 5), pp.1994-1999. ⟨10.1021/acsphotonics.7b01475⟩. ⟨hal-01777981⟩
297 Consultations
340 Téléchargements

Altmetric

Partager

More