Confinement and Time Immemorial: Prebiotic Synthesis of Nucleotides on a Porous Mineral Nanoreactor

We report the successful one-pot synthesis of adenosine mono-, di-, and triphosphate in the confined space of a mordenite zeolite. This is also the first report of ATP synthesized onto a porous mineral surface. The results revealed a plausible prebiotic route to ribonucleotides and highlighted the contribution of microporous minerals in the origins of life.

Mots clés

Mordenite RNA building blocks phosphoribosyl pyrophosphate ribonucleotides Origins of Life.

Domaines

Physique [physics]

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Accepted manuscript, HAL.pdf (791.04 Ko)

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https://hal.sorbonne-universite.fr/hal-02308428

Soumis le : mardi 8 octobre 2019-15:03:29

Dernière modification le : mercredi 28 août 2024-03:05:27

Dates et versions

hal-02308428 , version 1 (08-10-2019)

Identifiants

HAL Id : hal-02308428 , version 1
DOI : 10.1021/acs.jpclett.9b01448

Citer

Francisco Rodrigues, Thomas Georgelin, Guillaume Gabant, Baptiste Rigaud, Fabrice Gaslain, et al.. Confinement and Time Immemorial: Prebiotic Synthesis of Nucleotides on a Porous Mineral Nanoreactor. Journal of Physical Chemistry Letters, 2019, 10 (15), pp.4192-4196. ⟨10.1021/acs.jpclett.9b01448⟩. ⟨hal-02308428⟩

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